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A furan Diels–Alder cycloaddition approach to scyphostatin analogues†
Calum J. Fraser,Gareth P. Howell,Joseph P. A. Harrity
Organic & Biomolecular Chemistry Pub Date : 10/16/2012 00:00:00 , DOI:10.1039/C2OB26793D
Abstract

The synthesis of two diastereoisomers of the epoxycyclohexenone core of scyphostatin, a naturally occurring sphingomyelinase inhibitor, has been achieved via a common oxabicyclic intermediate. The diastereomeric intermediates are accessed by stereodivergent oxidative functionalisation processes, followed by a Lewis acid mediated ring opening rearrangement reaction.

Graphical abstract: A furan Diels–Alder cycloaddition approach to scyphostatin analogues
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