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The first use of methyl 2-pyridyl ketone oxime (mpkoH) in zinc(II)/lanthanide(III) chemistry leads to the [ZnLn(mpko)3(mpkoH)3](ClO4)2 and [ZnLn(NO3)2(mpko)3(mpkoH)] families of dinuclear ZnIILnIII complexes displaying blue-green, ligand-based photoluminescence; the ZnIIDyIII compound shows field-induced relaxation of magnetization.
