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E–H (E = R3Si or H) bond activation by B(C6F5)3 and heteroarenes; competitive dehydrosilylation, hydrosilylation and hydrogenation†
Liam D. Curless,Ewan R. Clark,Jay J. Dunsford,Michael J. Ingleson
Chemical Communications Pub Date : 11/29/2013 00:00:00 , DOI:10.1039/C3CC47372D
Abstract

In the presence of B(C6F5)3 five-membered heteroarenes undergo dehydrosilylation and hydrosilylation with silanes. The former, favoured on addition of a weak base, produces H2 as a by-product making the process catalytic in B(C6F5)3 but also enabling competitive heteroarene hydrogenation.

Graphical abstract: E–H (E = R3Si or H) bond activation by B(C6F5)3 and heteroarenes; competitive dehydrosilylation, hydrosilylation and hydrogenation
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