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Cu(i)-catalyzed tandem benzyldiazoester coupling with terminal alkyne–allene formation–Michael reaction: Application to the syntheses of oxa and azacycles†
Gullapalli Kumaraswamy,Neerasa Jayaprakash,Guniganti Balakishan
Organic & Biomolecular Chemistry Pub Date : 08/31/2011 00:00:00 , DOI:10.1039/C1OB06128C
Abstract

A simple and practical procedure for the synthesis of aza- and oxacycles, which possess an array of stereogenic functionalities, is described. This protocol relies on tandem Cu-catalyzed coupling of suitably functionalized terminal alkyne with diazoester followed by isomerization and subsequent aza or oxa-Michael reaction, thus generating the required scaffold with high diastereoselectivity.

Graphical abstract: Cu(i)-catalyzed tandem benzyldiazoester coupling with terminal alkyne–allene formation–Michael reaction: Application to the syntheses of oxa and azacycles
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