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Ellipticity controlled dissociative double ionization of ethane by strong fields
Gihan Basnayake,Paul Hoerner,Benoit Mignolet,Mi Kyung Lee,Yun Fei Lin,Alexander H. Winney,Duke A. Debrah,Leon Popaj,Xuetao Shi,Suk Kyoung Lee,H. Bernhard Schlegel,Francoise Remacle,Wen Li
Physical Chemistry Chemical Physics Pub Date : 10/08/2021 00:00:00 , DOI:10.1039/D1CP03585A
Abstract

The yields of all dissociation channels of ethane dications produced by strong field double ionization were measured. It was found that the branching ratios can be controlled by varying the ellipticity of laser pulses. The CH3+ formation and H+ formation channels show a clear competition, producing the highest and lowest branching ratios at ellipticity of ∼0.6, respectively. With the help of theoretical calculations, such a control was attributed to the ellipticity dependent yields of different sequential ionization pathways.

Graphical abstract: Ellipticity controlled dissociative double ionization of ethane by strong fields
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