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Fast and fully reversible photochromic performance of hybrid sol–gel films doped with a fused-naphthopyran
Paulo J. Coelho,Carlos J. R. Silva,Céu Sousa,Sandra D. F. C. Moreira
Journal of Materials Chemistry C Pub Date : 07/11/2013 00:00:00 , DOI:10.1039/C3TC31223B
Abstract

A new type of photochromic naphthopyran with a fused structure was embedded in an organic–inorganic aminealcohol–silicate hybrid gel producing colourless, transparent and flexible photochromic films. Under UV-vis light these materials developed, in less than 30 s, intense yellow-orange colours that faded completely in the dark in 3 min. This behaviour contrasts with the usual performance of common naphthopyrans that always generate two coloured species which fade with different kinetics, leading to the formation of a residual colour that persists for several minutes/hours. The structural design of this new naphthopyran prevents the formation of the long-lived coloured species and therefore fully reversible photo-switchable materials can be easily obtained.

Graphical abstract: Fast and fully reversible photochromic performance of hybrid sol–gel films doped with a fused-naphthopyran
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