Highly selective hydroformylation of long-chain alkenes in a supercritical fluid ionic liquid biphasic system†‡
Green Chemistry Pub Date : 05/26/2011 00:00:00 , DOI:10.1039/C1GC15142H
Abstract

Continuous-flow rhodium-catalysed hydroformylation of long chain alkenes has been achieved with selectivities to the desired linear aldehyde of 92% and minimum rhodium loss, using a xantphos-derived ligand attached to an imidazolium salt in a supercritical fluid–ionic liquid system. The effect of oxygen in the system can be ameliorated to some extent by adding a simple sulfonated triphenylphosphine to the catalytic solution.

Graphical abstract: Highly selective hydroformylation of long-chain alkenes in a supercritical fluid ionic liquid biphasic system