Highly enantioselective dynamic kinetic resolution and desymmetrization processes by cyclocondensation of chiral aminoalcohols with racemic or prochiral δ-oxoacid derivatives†
Mercedes Amat,Oriol Bassas,Miquel A. Pericàs,Mireia Pastó,Joan Bosch
Chemical Communications Pub Date : 01/20/2005 00:00:00 , DOI:10.1039/B413937B
Abstract

Cyclocondensation reactions of aminoalcohols 7 and 8 with racemic or prochiral δ-oxoacid derivatives provide polysubstituted lactams with high enantioselectivity in a process that involves dynamic kinetic resolution and/or desymmetrization of enantiotopic or diastereotopic ester groups.

Graphical abstract: Highly enantioselective dynamic kinetic resolution and desymmetrization processes by cyclocondensation of chiral aminoalcohols with racemic or prochiral δ-oxoacid derivatives