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A novel approach for the synthesis of imidazo and triazolopyridines from dithioesters†
Ajjahalli B. Ramesha,Nagarakere C. Sandhya,Chottanahalli S. Pavan Kumar,Mahanthawamy Hiremath,Kempegowda Mantelingu,Kanchugarakoppal S. Rangappa
New Journal of Chemistry Pub Date : 07/12/2016 00:00:00 , DOI:10.1039/C6NJ01038E
Abstract

T3P–DMSO mediated desulfurative cyclization of in situ generated thioamides serves as an efficient and versatile method for the synthesis of imidazo[1,5-a]pyridines and [1,2,4]-triazolo[4,3-a]pyridines with good to excellent yields. Substrates such as 2-methylaminoquinoline and pyrazin-2-yl-methanamine also undergo the corresponding reactions at room temperature. This efficient protocol has several advantages such as mild conditions, short reaction time, operational simplicity and high yields.

Graphical abstract: A novel approach for the synthesis of imidazo and triazolopyridines from dithioesters
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