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Manipulation and measurement of pH sensitive metal–ligand binding using electrochemical proton generation and metal detection†
Tania L. Read,Maxim B. Joseph,Julie V. Macpherson
Chemical Communications Pub Date : 12/08/2015 00:00:00 , DOI:10.1039/C5CC09326K
Abstract

Generator-detector electrodes can be used to both perturb and monitor pH dependant metal–ligand binding equilibria, in situ. In particular, protons generated at the generator locally influence the speciation of metal (Cu2+) in the presence of ligand (triethylenetetraamine), with the detector employed to monitor, in real time, free metal (Cu2+) concentrations.

Graphical abstract: Manipulation and measurement of pH sensitive metal–ligand binding using electrochemical proton generation and metal detection
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