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Metal-free visible-light-promoted C(sp3)–H functionalization of aliphatic cyclic ethers using trace O2†
Ben Niu,Bryan G. Blackburn,Krishnakumar Sachidanandan,Maria Victoria Cooke,Sébastien Laulhé
Green Chemistry Pub Date : 11/05/2021 00:00:00 , DOI:10.1039/D1GC03482K
Abstract

Presented is a light-promoted C–C bond forming reaction yielding sulfone and phosphate derivatives at room temperature in the absence of metals or photoredox catalyst. This transformation proceeds in neat conditions through an auto-oxidation mechanism which is maintained through the leaching of trace amounts of O2 as sole green oxidant.

Graphical abstract: Metal-free visible-light-promoted C(sp3)–H functionalization of aliphatic cyclic ethers using trace O2
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