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Novel monomers in radical ring-opening polymerisation for biodegradable and pH responsive nanoparticles†
Jenny Folini,Chao-Hung Huang,James C. Anderson,Wolfgang P. Meier
Polymer Chemistry Pub Date : 09/24/2019 00:00:00 , DOI:10.1039/C9PY01103J
Abstract

Responsive and biodegradable nanoparticles are essential for functional drug delivery systems. We herein report the first pH sensitive polyester from radical ring-opening polymerisation of novel amine-bearing cyclic ketene acetals (CKAs). The CKAs were synthesised via an intermediate carbonate and the resulting polyesters showed a pKa around pH 6. Together with an initial application in biodegradable nanoparticles, they open the pathway for a new generation of functional polyesters.

Graphical abstract: Novel monomers in radical ring-opening polymerisation for biodegradable and pH responsive nanoparticles
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