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Reaction of stannylene phosphorus Lewis pairs with dichlorides of germanium, tin and lead – the formation of base stabilized stannyl stannylenes/germylenes and redox reaction with PbCl2†
K. M. Krebs,J.-J. Maudrich,L. Wesemann
Dalton Transactions Pub Date : 04/14/2016 00:00:00 , DOI:10.1039/C6DT00916F
Abstract

The reaction of intramolecular stannylene phosphorus Lewis pairs with heavier dichlorides of group 14 (GeCl2, SnCl2, PbCl2) is reported. Phosphine base stabilized stannyl germylenes/stannylenes were formed by the oxidative addition of an E–Cl bond to the stannylene tin atom (E = Ge, Sn). In solution, a dynamic equilibrium between two diastereomeric configurations was observed. With PbCl2 a redox reaction towards elemental lead and the dichlorinated tin(IV) compound was found. All compounds were characterized by X-ray diffraction, NMR spectroscopy and elemental analysis.

Graphical abstract: Reaction of stannylene phosphorus Lewis pairs with dichlorides of germanium, tin and lead – the formation of base stabilized stannyl stannylenes/germylenes and redox reaction with PbCl2
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