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Recombinant oxalate decarboxylase: enhancement of a hybrid catalytic cascade for the complete electro-oxidation of glycerol†
Sofiene Abdellaoui,David P. Hickey,Andrew R. Stephens,Shelley D. Minteer
Chemical Communications Pub Date : 08/10/2015 00:00:00 , DOI:10.1039/C5CC06131H
Abstract

The complete electro-oxidation of glycerol to CO2 is performed through an oxidation cascade using a hybrid catalytic system combining a recombinant enzyme, oxalate decarboxylase from Bacillus subtilis, and an organic oxidation catalyst, 4-amino-TEMPO. This system is capable of electrochemically oxidizing glycerol at a carbon electrode collecting all 14 electrons per molecule.

Graphical abstract: Recombinant oxalate decarboxylase: enhancement of a hybrid catalytic cascade for the complete electro-oxidation of glycerol
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