Sorption enhanced CO2 methanation
Andreas Borgschulte,Noris Gallandat,Benjamin Probst,Riccardo Suter,Elsa Callini,Davide Ferri,Yadira Arroyo,Rolf Erni,Hans Geerlings,Andreas Züttel
Physical Chemistry Chemical Physics Pub Date : 04/15/2013 00:00:00 , DOI:10.1039/C3CP51408K
Abstract

The transformation from the fatuous consumption of fossil energy towards a sustainable energy circle is most easily marketable by not changing the underlying energy carrier but generating it from renewable energy. Hydrocarbons can be principally produced from renewable hydrogen and carbon dioxide collected by biomass. However, research is needed to increase the energetic and economic efficiency of the process. We demonstrate the enhancement of CO2 methanation by sorption enhanced catalysis. The preparation and catalytic activity of sorption catalysts based on Ni particles in zeolites is reported. The functioning of the sorption catalysis is discussed together with the determination of the reaction mechanism, providing implications for new ways in catalysis.

Graphical abstract: Sorption enhanced CO2 methanation