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Synthesis and characterization of a dipyriamethyrin–uranyl complex†
James T. Brewster, II,Qing He,Gonzalo Anguera,Matthew D. Moore,Xian-Sheng Ke,Vincent M. Lynch,Jonathan L. Sessler
Chemical Communications Pub Date : 04/12/2017 00:00:00 , DOI:10.1039/C7CC01674C
Abstract

The reaction between non-aqueous uranyl silylamide (UO2[N(SiMe3)2]2·2THF) under anaerobic conditions or uranyl acetate (UO2(OAc)2·2H2O) under standard laboratory conditions and dipyriamethryin affords a bench-stable uranyl complex. Competition studies as well as DFT calculations provide support for the observed selectivity for the uranyl cation over trivalent lanthanide and multiple transition metal precursors.

Graphical abstract: Synthesis and characterization of a dipyriamethyrin–uranyl complex
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