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Synthesis of tetraketones in water and under catalyst-free conditions†
Jian-Jun Yu,Li-Min Wang,Jin-Qian Liu,Feng-Lou Guo,Ying Liu,Ning Jiao
Green Chemistry Pub Date : 12/09/2009 00:00:00 , DOI:10.1039/B913816A
Abstract

A simple, environmentally friendly, tandem Knoevenagel condensation and Michael addition procedure is reported. The reactions between cyclic-13-diketones and a variety of aldehydes were carried out in water to afford tetraketones (64–99%). In this green synthetic protocol, the solvent water itself catalysed the reaction by hydrogen bonding, thus avoiding the use of any other catalysts to make the work up procedure easier.

Graphical abstract: Synthesis of tetraketones in water and under catalyst-free conditions
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