Synthesis of carbon-11 radiolabelled transition metal complexes using 11C-dithiocarbamates†,10.1039/D2DT00266C

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Synthesis of carbon-11 radiolabelled transition metal complexes using 11C-dithiocarbamates†

Sara Cesarec,Titan Lai,Christophe Plisson,Andrew J. P. White,Philip W. Miller

Dalton Transactions Pub Date : 03/10/2022 00:00:00 , DOI:10.1039/D2DT00266C

Abstract

A novel radiolabelling method exploiting ¹¹C-dithiocarbamate ligands has been used to generate ¹¹C-labelled Au(I), Au(III), Pd(II) and Pt(II) complexes in high radiochemical yields (71–99%). Labelled complexes were prepared in a rapid one-pot procedure via the substitution reaction of ¹¹C-dithiocarbamate ligands with appropriate transition metal chloride precursors.