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UV-induced modulation of the conductivity of polyaniline: towards a photo-patternable charge injection layer for structured organic light emitting diodes
Thomas Griesser,Archim Wolfberger,Matthias Edler,Andreas Pavitschitz,Markus Kratzer,Christian Teichert,Thomas Rath,Gregor Trimmel,Günther Schwabegger,Clemens Simbrunner,Helmut Sitter
Journal of Materials Chemistry Pub Date : 12/23/2011 00:00:00 , DOI:10.1039/C1JM14100G
Abstract

In macromolecular electronics the organic material should offer—besides the desired electronic properties—the possibility of lateral patterning. Here, we report on a novel polyaniline derivative bearing photosensitive N-formamide groups. UV illumination of this polymeric material leads to a decarbonylation reaction resulting in polyaniline which can be subsequently protonated to yield the conductive emeraldine salt. Due to the fact that the conductivity depends on the conversion of the photoreaction, a selective adjustment of the conductivity by means of UV light is feasible. These photo-induced conductivity changes were corroborated in thin films by conductive AFM measurements. Further, we demonstrate the versatility of this polymer with respect to a patterned modification of the conductivity as well as its application as a photo-patternable charge injection layer for structured OLEDs. This makes the new polymer an interesting candidate for electrodes and interconnects in various organic electronic devices.

Graphical abstract: UV-induced modulation of the conductivity of polyaniline: towards a photo-patternable charge injection layer for structured organic light emitting diodes
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