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Palladium-catalyzed cyclization of bromoenynamides to tricyclic azacycles: synthesis of trikentrin-like frameworks†
Craig D. Campbell,Rebecca L. Greenaway,Oliver T. Holton,Helen A. Chapman,Edward A. Anderson
Chemical Communications Pub Date : 08/22/2013 00:00:00 , DOI:10.1039/C3CC45634J
Abstract

Palladium-catalyzed cascade cyclization of bromoenynamides equipped with an additional alkyne or ynamide substituent affords azatricyclic products. Using 5- to 7-membered ring tethers, this chemistry offers a regiospecific route to highly-functionalized azacycles. Elaboration to the trikentrin B skeleton is achieved from the arylsilane cyclization products.

Graphical abstract: Palladium-catalyzed cyclization of bromoenynamides to tricyclic azacycles: synthesis of trikentrin-like frameworks
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