The first Td-symmetric lutetium metallofullerene, Lu2@C76, has been synthesized, isolated, and characterized. Because of the charge transfer from the encapsulated Lu atoms to the Td-C76 fullerene cage, the otherwise unstable Td-C76 fullerene can be significantly stabilized as a Lu2@C76 fullerene. Both STM and STS results are consistent with a charge state of (Lu2)6+@C766−(Td).