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Synthesis and solid state structure of a hydrazone-disulfidemacrocycle and its dynamic covalent ring-opening under acidic and basic conditions†
Max von Delius,Edzard M. Geertsema,David A. Leigh,Alexandra M. Z. Slawin
Organic & Biomolecular Chemistry Pub Date : 08/20/2010 00:00:00 , DOI:10.1039/C0OB00214C
Abstract

The synthesis and characterisation, including solid state structure, of a macrocycle containing both a hydrazone and a disulfide linkage is described. Selective ring-opening of the macrocycle under thermodynamic control could be achieved at either the disulfide or the hydrazone linkage by applying mutually exclusive sets of reaction conditions.

Graphical abstract: Synthesis and solid state structure of a hydrazone-disulfide macrocycle and its dynamic covalent ring-opening under acidic and basic conditions
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