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Porpholactams and chlorolactams: replacement of a β,β′-double bond in meso-tetraphenyl-porphyrin and -chlorin by a lactam moiety†‡§
Joshua Akhigbe,John Haskoor,Matthias Zeller,Christian Brückner
Chemical Communications Pub Date : 06/28/2011 00:00:00 , DOI:10.1039/C1CC12955D
Abstract

Reaction of meso-tetraphenylporpholactone with hydrazine converts the lactone moiety to an N-aminolactam. It also reduces the opposite pyrrolic moiety of both the starting material and the N-aminolactam, generating chlorin-like chlorolactone and N-aminochlorolactam, respectively. Reductive N–N cleavage of the N-aminoporpholactam generates the parent porpholactam.

Graphical abstract: Porpholactams and chlorolactams: replacement of a β,β′-double bond in meso-tetraphenyl-porphyrin and -chlorin by a lactam moiety
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